International Conference on Optics and Laser technology

October 24-25,2024 | Paris, France

Heterodyne laser correlation Spectroscopy: An interferometric method for measuring nanoparticle velocity

Eric Buhler

University Paris Cite, France

Biography :

Eric Buhler currently holds a Full Professor position in soft condensed matter physics at Universite Paris Cite (France). In 1996, he received his Ph.D. degree in physics at the University of Strasbourg investigating the struc­tural and dynamical properties of wormlike micelles. Prof. E. Buhler subsequently obtained a postdoctoral posi­tion (1996-1998) at the University of North Carolina at Chapel Hill (USA), where he studied the structural behavior of copolymers in supercritical carbon dioxide using scattering techniques. In 1998, he joined the University of Grenoble, France, where he obtained an Associate Professor position (1998-2006). He spent two years (2002- 2004) at the French National Research Center (CNRS) of Montpellier (Charles Coulomb Institute) as a Visiting Professor. In 2006, he joined the Universite Paris Cite, where he is currently a Full Professor. His research focuses on the structure and dynamics of complex systems. He is specialist in laser light, neutron and X-ray scattering as well as in photon correlation spectroscopy. He has published more than 80 research articles in peer review journals.

Abstract :

In a flowing solution of motorized nanoparticles, propelled objects undergo both directed flow and random diffusion, and equations for forced diffusion can be used to describe this sit­uation. Dynamic laser light scattering (DLS or photon correlation spectroscopy) is a well-es­tablished technique for measuring particle size over the size range from few nanometers to few micrometers and a technique of choice for studying the dynamics of solutions and in particular diffusive processes due to Brownian motion. However, the average drift velocity of particles, in a directed flow is inaccessible in a standard homodyne DLS experiments. The study of ballistic motions or forced diffusion requires advanced heterodyne DLS experiments. In such experiments a reference beam, which is a small fraction of the intensity of the inci­dent laser light, is mixed with the light scattered from the sample, allowing measurement of dynamical structure factors characterized by both real (diffusion) and complex (ballistic ve­locity) processes. Important. The heterodyne intensity-intensity correlation function, g(2)(q), is an oscillating function of the time lag with a velocity-dependent frequency that requires complex analyses and comparison with theoretical models. Such recent optical setup and method recently enabled us to study complex motions of active nanoparticles.